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SolvatochromicPhotoluminescentEffects inAll-InorganicManganese(II)-BasedPerovskites by HighlySelectiveSolvent-InducedCrystal… : научноеиздание Xiao HuiDang PeipeiYun Xiaohan2021 год

Solvatochromic Photoluminescent Effects in All-Inorganic Manganese(II)-Based Perovskites by Highly Selective Solvent-Induced Crystal-to-Crystal Phase Transformations : научное издание
статья из журнала

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База данных: Каталог библиотеки СФУ
Библиографическое описание: Solvatochromic Photoluminescent Effects in All-Inorganic Manganese(II)-Based Perovskites by Highly Selective Solvent-Induced Crystal-to-Crystal Phase Transformations : научное издание / H. Xiao, P. Dang, X. Yun [et al.]. - Текст : непосредственный // Angewandte Chemie. - 2021. - Т. 133, № 7. - P. 3743-3751. - ISSN 0044-8249. - ISSN 1521-3757, DOI 10.1002/ange.202012383.
Аннотация: <jats:title>Abstract</jats:title><jats:p>The development of lead-free perovskite photoelectric materials has been an extensive focus in the recent years. Herein, a novel one-dimensional (1D) lead-free CsMnCl<jats:sub>3</jats:sub>(H<jats:sub>2</jats:sub>O)<jats:sub>2</jats:sub> single crystal is reported with solvatochromic photoluminescence properties. Interestingly, after contact with N,N-dimethylacetamide (DMAC) or N,N-dimethylformamide (DMF), the crystal structure can transform from 1D CsMnCl<jats:sub>3</jats:sub>(H<jats:sub>2</jats:sub>O)<jats:sub>2</jats:sub> to 0D Cs<jats:sub>3</jats:sub>MnCl<jats:sub>5</jats:sub> and finally transform into 0D Cs<jats:sub>2</jats:sub>MnCl<jats:sub>4</jats:sub>(H<jats:sub>2</jats:sub>O)<jats:sub>2</jats:sub>. The solvent-induced crystal-to-crystal phase transformations are accompanied by loss and regaining of water of crystallization, leading to the change of the coordination number of Mn<jats:sup>2+</jats:sup>. Correspondingly, the luminescence changes from red to bright green and finally back to red emission. By fabricating a test-paper containing CsMnCl<jats:sub>3</jats:sub>(H<jats:sub>2</jats:sub>O)<jats:sub>2</jats:sub>, DMAC and DMF can be detected quickly with a response time of less than one minute. These results can expand potential applications for low-dimensional lead-free perovskites.</jats:p>
Год издания: 2021
Авторы: Xiao Hui , Dang Peipei , Yun Xiaohan , Li Guogang , Wei Yi , Wei Yi , Xiao Xiao , Zhao Yajie , Molokeev Maxim S. , Cheng Ziyong , Lin Jun
Издательство: John Wiley & Sons, Incorporated
Источник: Angewandte Chemie
Выпуск: Т. 133, № 7
Номера страниц: 3743-3751
Держатель оригинала документа: Department of Physics Far Eastern State Transport University 680021 Khabarovsk Russia, Engineering Research Center of Nano-Geomaterials of Ministry of Education Faculty of Materials Science and Chemistry China University of Geosciences Wuhan 430074 China, Laboratory of Crystal Physics Kirensky Institute of Physics Federal Research Center KSC SB RAS 660036 Krasnoyarsk Russia, Siberian Federal University 660041 Krasnoyarsk Russia, State Key Laboratory of Rare Earth Resource Utilization Changchun Institute of Applied Chemistry Chinese Academy of Sciences 5625 Renmin Street Changchun 130022 China, University of Science and Technology of China Hefei 230026 China
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