Rebuilding the vibrational wavepacket in TRAS using attosecond X-ray pulses : научное издание

Wang Chao; Gong Maomao; Zhao Xi; Nan Quan Wei; Yu Xin Yue; Cheng Yongjun; Kimberg Victor; Liu Xiao-Jing; Vendrell Oriol; Ueda Kiyoshi; Zhang Song Bin

Дополнительные ссылки: eLibrary

База данных: Каталог библиотеки СФУ

Библиографическое описание: Rebuilding the vibrational wavepacket in TRAS using attosecond X-ray pulses : научное издание / C. Wang, M. Gong, X. Zhao [et al.]. - Текст : непосредственный // Communications Physics. - 2024. - Т. 7, № 1. - P. 1. - ISSN 2399-3650. - ISSN 2399-3650, DOI 10.1038/s42005-023-01507-3.

Аннотация: AbstractTime-resolved X-ray photoelectron spectroscopy (TXPS) is a well-established technique to probe coherent nuclear wavepacket dynamics using both table-top and free-electron-based ultrafast X-ray lasers. Energy resolution, however, becomes compromised for a very short pulse duration in the sub-femtosecond range. By resonantly tuning the X-ray pulse to core-excited states undergoing Auger decay, this drawback of TXPS can be mitigated. While resonant Auger-electron spectroscopy (RAS) can recover the vibrational structures not hidden by broadband excitation, the full reconstruction of the wavepacket is a standing challenge. Here, we theoretically demonstrate how the complete information of a nuclear wavepacket, i.e., the populations and relative phases of the vibrational states constituting the wavepacket, can be retrieved from time-resolved RAS (TRAS) measurements. Thus, TRAS offers key insights into coupled nuclear and electronic dynamics in complex systems on ultrashort timescales, providing an alternative to leverage femtosecond and attosecond X-ray probe pulses.

Год издания: 2024

Авторы: Wang Chao, Gong Maomao, Zhao Xi, Nan Quan Wei, Yu Xin Yue, Cheng Yongjun, Kimberg Victor, Liu Xiao-Jing, Vendrell Oriol, Ueda Kiyoshi, Zhang Song Bin

Издательство: NATURE PUBLISHING GROUP, MACMILLAN BUILDING, 4 CRINAN ST, LONDON, ENGLAND, N1 9XW

Источник: Communications Physics

Выпуск: Т. 7, № 1

Номера страниц: 1

Количество экземпляров:

Твёрдая копия издания отсутствует в фонде библиотеки

Показать дополнительные сведения

Resonant Auger Scattering by Attosecond X-Ray Pulses : научное издание

Nan Quan-Wei и др.
2023 год

Selective gating to vibrational modes through resonant X-ray scattering : статья из журнала

Couto Rafael C. и др.
2017 год

Wave packet theory for non-resonant x-ray emission and non-resonant Auger electron emission in… : статья из журнала

Savchenko Viktoriia и др.
2023 год

Coincidence spectroscopy of molecular normal Auger decay by ultrashort x-ray pulses : научное издание

Zhu Yan Ping и др.
2022 год

Nonlinear resonant Auger spectroscopy in CO using an x-ray pump-control scheme : статья из журнала

Zhang Song Bin и др.
2016 год

X-ray transient absorption spectroscopy by an ultrashort x-ray-laser pulse in a continuous-wave IR… : научное издание

Shi Xin и др.
2020 год

Core-Excited Molecules by Resonant Intense X-Ray Pulses Involving Electron-Rotation Coupling : научное издание

Zhu Yanping и др.
2021 год

Suppression of resonant auger effect with chirped x-ray free-electron laser pulse : научное издание

Sun Y.-P. и др.
2018 год

Unveiling the X-ray-Induced Rabi Dynamics in Resonant Auger Fragment Spectra : научное издание

Nan Quan Wei и др.
2025 год

High-resolution x-ray spectra of carbon monoxide reveal ultrafast dynamics induced by long UV pulse : научное издание

Liu Ji-Cai и др.
2021 год

A study of the water molecule using frequency control over nuclear dynamics in resonant X-ray… : научное издание

Vaz da Cruz V. и др.
2017 год

Attosecond processes and X-ray spectroscopy: General discussion : научное издание

Milne C.J. и др.
2016 год

Probing hydrogen bond strength in liquid water by resonant inelastic X-ray scattering : научное издание

da Cruz Vinicius Vaz и др.
2019 год

Core-excited states of SF6 probed with soft-x-ray femtosecond transient absorption of vibrational… : научное издание

Barreau Lou и др.
2023 год

Parity violation in resonant inelastic soft x-ray scattering at entangled core holes : статья из журнала

Söderström Johan и др.
2024 год

Hydrogen bond effects in multimode nuclear dynamics of acetic acid observed via resonant x-ray… : статья из журнала

Savchenko Viktoriia и др.
2021 год

Библиотечно-издательский комплекс СФУ

Rebuilding the vibrational wavepacket in TRAS using attosecond X-ray pulses : научное издание
статья из журнала

Похожие публикации