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Sequential andReversible PhaseTransformations inZero-DimensionalOrganic-InorganicHybrid Sb-basedHalides towardsMultiple… : научноеиздание Li BohanJin JianceYin Meijuan2022 год

Sequential and Reversible Phase Transformations in Zero-Dimensional Organic-Inorganic Hybrid Sb-based Halides towards Multiple Emissions : научное издание
статья из журнала

Дополнительные ссылки: eLibrary
База данных: Каталог библиотеки СФУ
Библиографическое описание: Sequential and Reversible Phase Transformations in Zero-Dimensional Organic-Inorganic Hybrid Sb-based Halides towards Multiple Emissions : научное издание / B. B. Li [et al.]. - Текст : непосредственный // Angewandte Chemie. - 2022. - Т. 134, № 49. - ISSN 0044-8249. - ISSN 1521-3757, DOI 10.1002/ange.202212741.
Аннотация: <jats:title>Abstract</jats:title><jats:p>Zero-dimensional (0D) metal halides have drawn increasing attention due to the attractive structure dependent photoluminescence (PL) properties. Here, we report two new 0D organic–inorganic hybrid Sb-based halides, (MTP)<jats:sub>6</jats:sub>SbBr<jats:sub>6</jats:sub>Sb<jats:sub>2</jats:sub>Br<jats:sub>9</jats:sub>⋅H<jats:sub>2</jats:sub>O (MTP=Methyltriphenylphosphonium, crystal 1) and (MTP)<jats:sub>2</jats:sub>SbBr<jats:sub>5</jats:sub> (crystal 2), featuring a reversible structural phase transformation and tunable orange and red emissions upon dehydration and rehydration of H<jats:sub>2</jats:sub>O molecules. Intriguingly, a subsequent heat treatment further enables the formation of glassy state (MTP)<jats:sub>2</jats:sub>SbBr<jats:sub>5</jats:sub> (glass 3) with near-infrared luminescence, moreover, a sequential reverse phase transformation from glass 3 to crystal 2 and 1 is triggered by acetonitrile and water vapor stepwise. The anti-counterfeiting demo based on the tunable and reversible PL switching is finally achieved and thus the phase structure engineering in 0D metal halides expands their multiple applications in optical fields.</jats:p>
Год издания: 2022
Авторы: Li Bohan , Jin Jiance , Yin Meijuan , Zhang Xinlei , Molokeev Maxim S. , Xia Zhiguo , Xu Yan
Издательство: John Wiley & Sons
Источник: Angewandte Chemie
Выпуск: Т. 134, № 49
Держатель оригинала документа: Department of Chemistry College of Sciences Northeastern University Shenyang Liaoning 110819 China, Department of Physics Far Eastern State Transport University Khabarovsk 680021 Russia, Laboratory of Crystal Physics Kirensky Institute of Physics Federal Research Center KSC SB RAS Krasnoyarsk 660036 Russia, School of Physics and Optoelectronics State Key Laboratory of Luminescent Materials and Devices South China University of Technology Guangzhou 510641 China, Siberian Federal University Krasnoyarsk 660041 Russia
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